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Photon-echo spectroscopy with 5-fs pulses

Maxim S. Pshenichnikov, Andrius Baltuška, and Douwe A. Wiersma

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Abstract

The formalism for transient photon-echo spectroscopy with extremely short laser pulses that consist of only a few optical cycles is discussed. The pure dephasing time of the hydrated electron is measured as ~1.6 fs which is consistent with the absorption line width.

© 2000 Optical Society of America

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