Direct Evidence of Ultrafast Energy Delocalization in a Strongly Coupled Organic Microcavity probed by Two-Dimensional Electronic Spectroscopy

Mattia Russo; Kyriacos Georgiou; Kyriacos Georgiou; Armando Genco; Simone De Liberato; Giulio Cerullo; David G. Lidzey; Andreas Othonos; Margherita Maiuri; Tersilla Virgili

doi:10.1364/UP.2022.M2A.7

The International Conference on Ultrafast Phenomena (UP) 2022
Technical Digest Series (Optica Publishing Group, 2022),
paper M2A.7
•https://doi.org/10.1364/UP.2022.M2A.7

Direct Evidence of Ultrafast Energy Delocalization in a Strongly Coupled Organic Microcavity probed by Two-Dimensional Electronic Spectroscopy

Mattia Russo, Kyriacos Georgiou, Armando Genco, Simone De Liberato, Giulio Cerullo, David G. Lidzey, Andreas Othonos, Margherita Maiuri, and Tersilla Virgili

International Conference on Ultrafast Phenomena 2022

Montreal, Quebec Canada
18–22 July 2022
ISBN: 978-1-957171-07-4

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Femtochemistry (M2A)

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M. Russo, K. Georgiou, A. Genco, S. De Liberato, G. Cerullo, D. G. Lidzey, A. Othonos, M. Maiuri, and T. Virgili, "Direct Evidence of Ultrafast Energy Delocalization in a Strongly Coupled Organic Microcavity probed by Two-Dimensional Electronic Spectroscopy," in The International Conference on Ultrafast Phenomena (UP) 2022, F. Légaré, T. Tahara, J. Biegert, T. Brixner, and N. Dudovich, eds., Technical Digest Series (Optica Publishing Group, 2022), paper M2A.7.

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Abstract

Two-Dimensional Electronic Spectroscopy reveals an ultrafast energy delocalization between 2μm distanced donor/acceptor molecules confined in a microcavity. This mechanism is promoted by the formation of hybrid-polariton states that induces a coupling in the entire system.

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