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Polarization control of rotationally-resolved 2D infrared spectroscopy

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Abstract

Recent technological developments are enabling highly sensitive measurements of high-resolution 2D IR gas-phase spectra. In analogy to well-known liquid-phase results, we present polarization sequences that reduce spectral congestion and improve signal separation in gas-phase spectra. We also discuss other unique features of 2DIR gas phase spectra.

© 2022 The Author(s)

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