Abstract

This paper proposes a new form of nonsteady-state anti-Stokes near-field spectroscopy with high spatial resolution in Dicke's optical superradiation regime. A system of kinetic equations is constructed that describes collections of excited atoms and fluorescence photons in the far field. It is solved approximately, and a formula is obtained for the signal intensity of nonsteady-state anti-Stokes near-field spectroscopy. Possible ways of constructing a new method of high-spatial-resolution spectroscopy of atoms and molecules are discussed.

A scheme for detecting the atom-field coupling constant in the Dicke superradiation regime using hybrid cavity optomechanical system

Yueming Wang, Bin Liu, Jinling Lian, and Jiuqing Liang
Opt. Express 20(9) 10106-10114 (2012)

Superradiance of non-Dicke states

N. E. Nefedkin, E. S. Andrianov, A. A. Zyablovsky, A. A. Pukhov, A. P. Vinogradov, and A. A. Lisyansky
Opt. Express 25(3) 2790-2804 (2017)

Scanning near-field optical coherent anti-Stokes Raman microscopy (SNOM-CARS) with femtosecond laser pulses in vibrational and electronic resonance

Mahesh Namboodiri, Tahir Zeb Khan, Sidhant Bom, Günter Flachenecker, and Arnulf Materny
Opt. Express 21(1) 918-926 (2013)

Near-field effects on coherent anti-Stokes Raman scattering microscopy imaging

Cheng Liu, Zhiwei Huang, Fake Lu, Wei Zheng, Dietmar W. Hutmacher, and Colin Sheppard
Opt. Express 15(7) 4118-4131 (2007)

Background-free coherent anti-Stokes Raman spectroscopy near transverse interfaces: a vectorial study

David Gachet, Franck Billard, and Hervé Rigneault
J. Opt. Soc. Am. B 25(10) 1655-1666 (2008)