Abstract
What we believe is a new scheme for producing semidiscrete self-trapped vortices (“swirling photon droplets”) in photonic crystals with competing quadratic (χ(2)) and self-defocusing cubic (χ(3)) nonlinearities is proposed. The photonic crystal is designed with a striped structure, in the form of spatially periodic modulation of the χ(2) susceptibility, which is imposed by the quasi-phase-matching technique. Unlike previous realizations of semidiscrete optical modes in composite media, built as combinations of continuous and arrayed discrete waveguides, the semidiscrete vortex “droplets” are produced here in the fully continuous medium. This work reveals that the system supports two types of semidiscrete vortex droplets, viz., onsite- and intersite-centered ones, which feature, respectively, odd and even numbers of stripes, $\mathcal {N}$. Stability areas for the states with different values of $\mathcal {N}$ are identified in the system’s parameter space. Some stability areas overlap with each other, giving rise to the multistability of states with different $\mathcal {N}$. The coexisting states are mutually degenerate, featuring equal values of the Hamiltonian and propagation constant. An experimental scheme to realize the droplets is outlined, suggesting new possibilities for the long-distance transmission of nontrivial vortex beams in nonlinear media.
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1. Introduction
Semidiscrete vortex quantum droplets, a new type of vortices, were initially predicted in binary Bose-Einstein condensates trapped in an array of tunnel-coupled quasi-1D potential wells [1]. Unlike vortex modes in fully continuous or fully discrete systems [2–7], these are stripe-shaped localized states, which are continuous in one direction and discrete in the perpendicular one, and do not exhibit rotational symmetry. It is well known that the stability of self-trapped vortex modes in two-dimensional (2D) and three-dimensional (3D) geometries is a challenging problem because the self-attractive nonlinearity gives rise to strong splitting instability of vortex rings and tori, even if the collapse instability that affects fundamental (zero-vorticity) solitons in the same media may be suppressed [8–13]. Due to the competition between the mean-field (MF) and beyond-MF effects in the bosonic condensate [14–23], semidiscrete vortex quantum droplets may maintain stability in this setting against the azimuthal (splitting) perturbations. The droplets exhibit significant differences from traditional solitons. The droplet state features a flat-top structure, characterized by an almost constant density distribution, bounded by relatively sharp edges. In the field of nonlinear optics, somewhat similar objects in the form of “photon droplets" were experimentally demonstrated in optical media with nonlocal (thermal) nonlinearity [24,25]. Actually, the competition between different nonlinear terms is a common effect [26–32], which occurs in the propagation of high-power laser beams in various media [32,33]. Optical semidiscrete vortex droplets can be maintained by the balance between the competing nonlinearities. In particular, stable self-bound semidiscrete vortex modes in the spatial domain were predicted in coupled planar waveguides with the cubic-quintic nonlinearity [34]. Similarly, self-bound spatiotemporal vortex modes can be predicted in coupled arrays of nonlinear fibers [35].
Recently, patterned quasi-phase matched (QPM) nonlinear photonic crystals in the 3D space have been produced by means of the thermoelectric field polarization [36], laser erasing [37], and femtosecond laser poling technique [38], which provides more possibilities for the creation of vortex states. The QPM technique has developed to a well-known method for achieving accurate phase matching in $\chi ^{(2)}$ crystals for the nonlinear frequency conversion [39–49] and nonlinear beam shaping [50–57] in different dimensions. Very recently, stable vortex solitons were predicted in 3D QPM photonic crystals [58]. The structure of the vortex solitons can be engineered by fixing different phase-matching conditions in different cells of the photonic crystals, thus inducing effective discreteness in this 3D optical medium. This technique offers a possibility of building semidiscrete vortex modes in the QPM-structured bulk photonic crystals. If the input power of the light field increases up to tens of GW/cm$^2$, third-order nonlinear effects are excited [32,33]. However, if one aims to induce fifth-order nonlinear effects, as demonstrated in Ref. [28], a higher power or a careful selection of specific optical materials is necessary.
The objective of this work is the construction of semidiscrete vortex optical droplets. This type of nontrivial self-bound vortices are able to yield more detailed information compared to the vortex self-localization solitons outlined in Ref. [27]. It is relevant to mention that effective 2D (but not 3D) discrete waveguiding structures for optical beams with the extraordinary polarization can be induced by means of a different technique in photorefractive materials illuminated by interfering beams with the ordinary polarization [59]. Such virtual photonic lattices were used for the creation of quasi-discrete 2D vortex solitons [60–62].
In this paper, we propose a scenario for the creation of semidiscrete vortex optical droplets in 3D photonic crystals with quadratic ($\chi ^{(2)}$) and defocusing cubic ($\chi ^{(3)}$) nonlinearities and a striped QPM-induced spatial structure, as shown in Fig. 1(a,b,c). As mentioned above, the $\chi ^{(3)}$ nonlinearity is able to compete with the $\chi ^{(2)}$ interaction if intensities of the light fields reach the level of several GW/cm$^{2}$ [32], making it possible to create self-bound photon droplets. We demonstrate that the phase-matching condition, adjusted to the striped structure, induces effective discreteness between adjacent stripes, which is necessary for the design of semidiscrete states. The balance of the competition between quadratic and cubic nonlinearity allows the self-bound vortex modes to maintain their stability.
The subsequent material is arranged as follows. The model is introduced in Section 3. Numerical results and estimates for the experimental setup are presented in Section 4. The paper is concluded by Section 5.
2. Model
The paraxial propagation of light beams through the 3D QPM photonic crystals with the competing $\chi ^{(2)}$ and $\chi ^{(3)}$ nonlinearities is governed by coupled equations for the slowly varying fundamental frequency (FF) and second harmonic (SH) amplitudes, $A_{1}$ and $A_{2}$:
Eq. (1), which keep, as said above, the terms with $m=\pm 1$ in Eq. (4), are simplified to the form of
Equations (6) and (7) conserve two dynamical invariants, viz., the Hamiltonian and total power (alias the Manley-Rowe invariant [68–70]):
3. Results
3.1 Numerical results
Stationary solutions to Eqs. (6) and (7) with propagation constant $\beta$ were looked for as
where $\phi _{1,2}$ are the stationary amplitudes of the FF and SH components. Vortex solutions were generated by means of the imaginary-time (imaginary-$z$) method, applied to Eqs. (6) and (7), with the input taken at $z=0$ asThe stability of the stationary vortex droplets was tested by direct real-$z$ simulations (through the algorithm of split-step Fourier transformation) of the perturbed evolution in the framework of Eqs. (6) and (7) up to $z=10000$. If the intensity pattern of the droplet remains unchanged up to this length (which corresponds to several diffraction lengths), it is categorized as a stable solution. Unstable solutions readily exhibit splitting in the course of the simulations.
As the stripe modulation acts solely in the $x$-direction, the vortex solutions feature similar modulation in the same direction and can be characterized by the number of stripes, $\mathcal {N}$, in the localized solution. According to Eq. (3), the solutions are also categorized into the OC and IC types. For the OC- and IC-type solutions, with the pivot located at the center of a stripe or at the border between adjacent stripes, numbers $\mathcal {N}$ are, respectively, odd or even. Typical examples for the OC-type vortex solution with $\mathcal {N}=3,5,7,9$ and IC-type ones with $\mathcal {N}=2,4,6,8$, all carrying the winding number $S=1$ in their FF component, are shown, respectively, in Figs. 2 and 3. These states feature a flat-top density structure, due to the competition between the quadratic and cubic nonlinear terms, which is a characteristic feature of droplet patterns. All these states are stable, as confirmed by direct simulations up to $z=10000$. Because the modulation is applied only along the $x$-direction, the vortex solutions feature a typical semidiscrete configuration similar to that reported in previous works [1,34]. However, unlike those works, the stable vortex modes are elaborated here in the bulk crystals with the spatially modulated local $\chi ^{(2)}$ susceptibility. In Fig. 1 (a), black and gray stripes represent positive and negative polarizations, respectively. Consequently, the density distribution of optical droplets at these positions on the x-axis induces a phase difference of $\pi /2$ in the second harmonic, leading to a quasi-discrete structure of the field. The vortex phase patterns exhibited in Figs. 2 and 3 of the SH component are striped to obey the matching condition of Eq. (14), hence, the effective angular coordinate of this component is defined by Eq. (13), showing a complicated striped-mixed vorticity pattern of this component.
Stability areas for the vortex solutions of the OC and IC types, with different values of $\mathcal {N}$ are shown, in the $(P,\ell )$ plane with $\Omega =0$ and $S=1$, in Fig. 4(a,b). These plots demonstrate that the vortex solutions with larger values of $P$ and smaller values of $\ell$ produce overlaps between different stability areas [see the cyan and yellow areas in Fig. 4(a), and the cyan area in Fig. 4(b)]. The overlaps indicate the presence of multistability in the system. To further illustrate this feature, we select $\ell =10$ and examine solutions with different values of $\mathcal {N}$, up to $P=200$. In this region, we find that four different values of $\mathcal {N}$ stably coexist at $P=200$ for both OC and IC types of solutions. Note also that the solutions with larger values of $\mathcal {N}$ require larger values of $P$ to support the stability. Multistable semidiscrete vortex solutions are characterized by values of $H$, $\beta$ and $r$, which are displayed, as functions of $P$, in Fig. 5, while keeping $\ell$ and $\Omega$ fixed. Notably, curves $H(P)$ and $\beta (P)$ for these solutions overlap almost completely, indicating degenerate solutions. The nearly flat dependences, with $d\beta /dP\approx 0$, indicate the existence of broad states, which may be considered as effectively liquid ones, cf. Reference [14]. A nearly constant value $r(P)\approx 2.7$ in Fig. 4(e,f) implies the domination of the FF component in the system. It is necessary to point out that the number of stripes, $\mathcal {N}$, is not a parameter affecting the droplet´s stabilization and multistability. Rather, this number distinguishes OC and IC (onsite- and intersite-centered) type solutions and to characterizes coexisting states. The key factors affecting the droplet’s stabilization and multistability are the total power ($P$) and period ($\ell$).
Finally, the phase-mismatch factor is determined by the modulation period $\Lambda$ (after the normalization, the phase mismatch exhibits by the effective detuning ´$\Omega$´). In Fig. 6 we present the range of the effective detuning for a fixed total power, $P=100$. The results indicate that stable semidiscrete vortex droplets exist for $\Omega \neq 0$.
Exploring vortex states with $S>1$ is a challenging problem, as they may be stable only for sufficiently large values of $P$. Two typical examples of stable vortex solutions of the OC and IC types with $S=2$, and $\mathcal {N}=5$ and $6$, are shown in Fig. 7. The stable solution with $S=2$ exists at $P>280$. This threshold is much higher than its counterpart for $S=1$, in which case the stable solutions are found at $P>40$.
3.2 Outline of the experimental setup
The fabrication of 3D photonic crystal by means of femtosecond laser pulses is a mature technology [71,72]. To estimate parameters of the setting under the consideration, we consider the nonlinear photonic crystal implemented in LiNbO$_{3}$, which has the second-order nonlinearity coefficient $d_{0}=d_{22}=2.1$ pm/V [73], and the third-order one $\chi ^{(3)}=6.6\times 10^{-22}$ m$^{2}$/V$^{2}$ [74]. The wavelengths of the FF and SH components are selected as $1064$ nm and $532$ nm, respectively. The relations between the scaled units, in which Eqs. (6) and (7) are written, and their physical counterparts can be established by means of Eq. (5), as summarizes in Table 1.
According to the results of the simulations (see Figs. 2 and 3), the peak droplet’s intensity in the FF and SH components are $I_{\mathrm {FF}}\approx 4.32$ GW/cm$^{2}$ and $I_{\mathrm {SH}}\approx 0.432$ GW/cm$^{2}$, respectively. If we select the pulse width as $200$ ps, the energy densities for the FF and SH components are $0.86$ J/cm$^{2}$ and $0.086$ J/cm$^{2}$, which are lower than the damage threshold ($\sim$1.5 J/cm $^{2}$ [75,76]) of the PPLN crystals. The characteristic propagation distance, which is $z=10000$, amounts to $2.8$ m, which is several times the underlying diffraction length. Therefore, the stability of the droplets, predicted by the simulations, is a reliable prediction.
The sketch for the experimental observation of these droplets is shown in Fig. 1(d): A high-power sub-nanosecond laser (e.g., one with the power exceeding $0.6$ mJ per pulse, $200$ ps pulse width, and $400$ Hz repetition rate) may be a suggested light source in the proposed experiment. The input patterns on the front surface of the PPLN can be generated by a spatial light modulator (SLM) and a Lens. Input FF and SF components can be selected with energies $0.37$ mJ and $0.16$ mJ per pulse, which are close to the FF/SF power ratio $r\approx 2.7$ for stationary semidiscrete vortex droplets in Figs. 6(e) and (f). If the input’s power ratio is essentially different from this value, it naturally gives rise to strong oscillations between the FF and SH components. The power and phase patterns of the FF component of the input, which are shown in the left inset of Fig. 1(d), can be produced by a properly designed SLM1 and L1, and the input SH patterns with $0.14$ mJ per pulse can be produced by SLM2 and L2, respectively. The FF and SH beams are coupled by the dichroic mirror, which sends them onto the PPLN coaxially. The necessary PPLN crystal may be $4$ cm long along the axial direction. Finally, the beams transmitted through the PPLN are imaged on to a camera by Lens L3. The simulated output patterns at the back surface of the crystals are shown in the right inset in Fig. 1(d).
4. Conclusion
We have proposed 3D photonic crystals with the striped structure and the combination of the $\chi ^{(2)}$ and defocusing $\chi ^{(3)}$ nonlinearities. The results of the analysis predict the creation of two types of stable semidiscrete vortex solutions, OC and IC (onsite- and intersite-centered ones), which exhibit an odd or even number of stripes in their structure, respectively. The smallest number of the stripes is $\mathcal {N}_{\text {OC}}=3$ or $\mathcal {N}_{\text {IC}}=2$. The setting admits with different numbers of stripes for the same parameters. Unlike the multistability in systems with the competing cubic-quintic nonlinear interactions, the Hamiltonian and propagation constant of these coexisting states are equal, thus featuring degeneracy. The range of the multistability has been found. The stable solutions for semidiscrete vortices exist within a certain range of positive or negative values of the phase mismatch of the $\chi ^{(2)}$ interaction in the medium.
The scheme proposed in this paper can be developed in other settings, such as photonic crystals with ring- or fan-shaped structures. Those settings can be used, in particular, for the implementation of various scenarios of beam shaping. It is worth noting that it is feasible to generalize the model introduced in this paper to include the sum-frequency generation and three-wave mixing by quadratic terms. In particular, it is relevant to analyze how soliton states change into droplets under the action of the three-wave mixing. Moreover, Furthermore, as detailed in Ref. [28], the ability to generate distinctive vortex self-localized states, such as ones with hidden vorticity, can be considered in the process of three-wave mixing. These findings are expected to extend into the investigation of vortex states in the realm of structured light fields [77,78].
Funding
National Natural Science Foundation of China (11874112, 12274077); Israel Science Foundation (1695/22); Ciuangdong-Hong Kong-Macao Joint l.aboratory for lntelligent Micro-Nano Optoelectroniclechnology (2020B1212030010).
Acknowledgment
Xiaoxi Xu and Feiyan Zhao, appreciate the Graduate Innovative Talents Training Program of Foshan University.
Disclosures
The authors declare no conflicts of interest.
Data availability
Data underlying the results presented in this paper are not publicly available at this time but may be obtained from the authors upon reasonable request.
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