Abstract
We derive generalized sheet transition conditions (GSTCs) including dipoles and quadrupoles, using generalized functions (distributions). This derivation verifies that the GSTCs are valid for metasurfaces in non-homogeneous environments, such as for practical metasurfaces fabricated on a substrate. The inclusion of quadrupoles and modeling of spatial dispersion provides additional hyper-susceptibility components which serve as degrees of freedom for wave transformations. We leverage them to demonstrate a generalized Brewster effect with multiple angles of incidence at which reflection is suppressed, along with an “anti-Brewster” effect where transmission is suppressed.
© 2023 Optica Publishing Group under the terms of the Optica Open Access Publishing Agreement
1. Introduction
The study of metamaterials, and metasurfaces in particular, has reached a level of maturity such that recent works present increasingly elaborate applications. While at first, metasurfaces were used to provide simple wave transformations [1,2] and flat optics [3], they have now been used for sophisticated holography [4] and recently for computation and signal processing [5–9]. This last application – where transfer functions are implemented in the Fourier domain – has required intricate design of meta-atoms to achieve control of the angular scattering response [9–11].
To aid in the design of metasurfaces for these applications, several modeling techniques have established themselves [12]. One popular approach is to model a metasurface as an impedance sheet which supports electric and magnetic currents [12–14]. This induces boundary conditions on the tangential parts of the electric and magnetic fields. However, the impedances do not provide characteristic parameters to represent the metasurface since they depend on the incident fields [15]. A second approach is to determine the polarizability of an isolated meta-atom and account for its coupling through the array to other meta-atoms using Green’s functions in the so-called T-matrix approach [16]. This provides insights into the multipole moments which are present, and how they couple together. However, it does not serve as a boundary condition; rather, it provides the scattered fields when the incident field is specified. The last popular approach is the use of surface susceptibilities, which represent the metasurface as a zero-thickness sheet of multipole moment densities [17–21]. Given these moments along a surface, generalized sheet transition conditions (GSTCs) provide boundary conditions on the fields adjacent to the surface [22]. These have been used to design metasurfaces [23] and also implemented in numerical methods to greatly decrease the computational resources needed for their analysis [24–26].
Recently, it has become evident that susceptibility modeling, which was previously limited to the dipolar regime, should include spatial dispersion (nonlocality) [27]. This was analyzed with “angle-dispersive” dipolar susceptiblities in [28] while we considered higher-order multipoles in [29,30]. These considerations are especially true for optical metasurfaces, which generally have large meta-atoms with dimensions that approach the wavelength. Using GSTCs that were generalized to include quadrupoles, we demonstrated an improvement in the modeling accuracy [30]. In addition to improving the accuracy, the additional susceptibility components provide additional degrees of freedom for designing metasurfaces.
However, the derivations in [30] are limited since they assume the media below and above the metasurface to be identical. Thus, it is not a priori obvious whether they would rigorously apply to practical metasurfaces which are usually fabricated on a substrate. In this work, we overcome the limitation of [30] by deriving the GSTCs, but using a different approach based on distributions (generalized functions) [31], inspired by the work of Idemen [32]. Ultimately, our derivation produces GSTCs identical to those in [30], which demonstrates that the latter can indeed be used in the presence of a substrate.
To demonstrate the utility of these GSTCs, we demonstrate the full control of the Brewster angle, where reflection at a dielectric interface is suppressed at a particular angle. By placing a metasurface at the dielectric interface, it is possible to tune the Brewster angle, as shown in [33,34]. We now leverage the higher-order susceptibility components to show that the additional degrees of freedom allow for further control, such as multiple Brewster angles, and suppression of transmission at particular angles—which we call “anti-Brewster” angles.
This paper is outlined as follows. First, we introduce generalized functions and derive the GSTCs in Section 2. Next, Section 3. presents considerations to enforce the physicality of the analysis: spatial dispersion, properties of the moment tensors, and spatial symmetries of meta-atoms. Then, several examples of controlling the Brewster and “anti-Brewster” angles are presented in Section 5. Finally, we conclude in Section 6.
2. GSTCs with quadrupoles
In this section, we will generalize the GSTCs to account for quadrupolar moments. Such a derivation was performed in [30], but with a caveat: the derivation assumed the bulk media adjacent to the metasurface to be homogeneous, and identical on both sides. This limitation arose from the use of the vector potential of the surface currents. We will overcome this limitation using an alternative derivation which represents the fields using distributions (generalized functions), following the approach taken by Idemen [32]. Using this approach, the bulk material properties can be arbitrary as they are embedded in the definitions of the fields. Nevertheless, it should be noted that the following developments are valid only if the metasurface is homogenizable, i.e., that its electromagnetic response can be expressed via effective material parameters. For this to be the case, the period of the metasurface array must be smaller than $\lambda _0 / (n_\text {i} + n_\text {s})$, where $\lambda _0$ is the wavelength in vacuum and $n_\text {i}$ and $n_\text {s}$ are the refractive indices of the incidence and scattering media, to prevent the existence of diffraction orders even up to grazing angles [35].
Distributions are ideal for modeling metasurfaces as zero-thickness discontinuities, since they formalize the notion of an “impulse function”. For example, the electric polarization of a flat metasurface in the $xy$ plane may be expressed as $\mathbf {P}(x,y,z)=\mathbf {P}'(x,y)\delta (z)$, where $\delta (z)$ is the Dirac delta distribution, which in turn is rigorously defined using test functions [32]. More generally, any field quantity $\Lambda$ can be decomposed into a continuous part and a discontinuous part:
where $\{\Lambda (z)\}$ represents the continuous part of $\Lambda (z)$ and a summation of the Dirac distribution and its derivatives is used to represent the discontinuity, as in Fig. 1. By interpreting Maxwell’s equations with all field quantities as distributions, discontinuities in the fields are acceptable and treated rigorously, one arrives at a new set of equations called the universal boundary conditions [32,36].The starting point to derive the GSTCs are the universal boundary conditions and the following relations for the electric and magnetic flux densities for media with multipolar responses [29,37]:
Naturally, these simplify to the conventional textbook boundary conditions for a dielectric interface when there are no surface polarization moments, which can be easily verified by setting $\mathbf {P}=\mathbf {M}=\overline {\overline {Q}}=\overline {\overline {S}}=0$.
3. Non-local considerations
The GSTCs (4 provide boundary conditions, but do not model how the polarization densities arise. These can be captured using multipolar susceptibilities. In this section, we formulate constitutive relations, and discuss some considerations that must be taken when the metasurface is placed in a non-uniform environment.
3.1 Acting fields
The fields which excite the meta-atoms are defined as the average of the adjacent fields on either side of the metasurface. As in [30,35,38], these average fields are usually defined as
This works well if the metasurface is freestanding, but is inappropriate if the metasurface is placed between two different media. Considering a thin slab placed between two different media, it can be shown (see Supplement 1 or [39]) that the normal components should be defined using the flux densities, $\epsilon E_{z}$ and $\mu H_{z}$, which remain continuous at a dielectric interface, such that the acting fields are
3.2 Spatial dispersion
Given the acting fields (6), the constitutive relations can be written out. If the metasurface response may be described in terms of only dipolar components (e.g., when the metasurface unit cell is much smaller than the wavelength so that higher-order multipolar components are negligible), the induced moments are related using [23,30]
Compared to (7), the extended constitutive relations (8) now include not only dipolar and quadrupolar responses but also their dependence on the fields and the gradients of the fields so as to account for higher-order spatially dispersive (nonlocal) effects. Interestingly, note that the quadrupolar susceptibilities that depend on the fields directly (e.g., $Q_{il}\propto Q_\text {ee}^{ilj}E_{\text {av},j}$) happen to be reciprocally connected to the dipolar components that depend on the field gradients (e.g., $P_{i}\propto \chi _\text {ee}^{'ijk}\nabla _k E_{\text {av},j}$) such that $Q_\text {ee}^{ilj}=\chi _\text {ee}^{'jli}$ and so on for the other hyper-susceptibility tensors [29]. At this point, for simplicity but without loss of generality, we will consider TM-polarized plane-wave fields propagating in the $xz$ plane. Then, as shown in [30], (8) simplifies to
First, consider Faraday’s equation in either medium, $\nabla \times \mathbf {E}=j\omega \mathbf {B}$, which becomes $\partial _zE_x=\partial _xE_z-j\omega B_y$. Then, it follows that the spatial average of the derivative along $z$ of $E_x$ may be obtained as
Finally, consider Ampere’s equation, $\nabla \times \mathbf {H}=j\omega \mathbf {D}$; that is, $\partial _zH_y=\partial _yH_z-j\omega D_x$.
Now, with reference to (10), (9) is modified to
3.3 Tensor symmetries, tracelessness, and reciprocity
Linear time-invariant metasurfaces that are not biased by a time-odd quantity (such as a magnetic field) are reciprocal and as such must satisfy reciprocity conditions [40,41]. Furthermore, we note that all of the moments should be symmetrical; e.g., $Q_{ij}=Q_{ji}$ [42]. These symmetry and reciprocity properties of the moments constrain the susceptibility terms such that they are related to one another as shown in [29]. Enforcing these relations reduces the 64 terms in Fig. 2(a) to 36.
In addition to being symmetrical, the tensors should be traceless. Only if this is the case are the moments truly physically meaningful, and are called irreducible [42,43]. In particular, note that $\sum _iQ_{ii}=0$, which implies $Q_{zz}=-Q_{xx}$ given that $Q_{yy}=0$ in our simplified problem. In contradiction to this condition, $Q_{zz}$ and $Q_{xx}$ are independent in (11).
To enforce tracelessness, note how the 6th row in Fig. 2(a) should be the negative of the 5th row ($Q_{zz}=-Q_{xx}$), and can thus be eliminated. However, reciprocity must still be enforced: the 5th row and 5th column are related by reciprocity and tensor symmetries. Given the relationship between the 4th and 5th rows, reciprocity is maintained by rewriting the 5th column as the negative of the 4th column. Then, the 5th row can be eliminated and we arrive at the $7\times 8$ matrix in Fig. 2(b). This matrix ensures tensor symmetries, reciprocity, and traceless, and contains 28 unique terms. After eliminating $Q_{zz}$, (11) becomes
3.4 Spatial symmetries
Neumann’s principle states that the material parameters of a system should exhibit the same symmetry properties as the physical structure they describe. This implies that if the considered physical structure (metasurface) is invariant under certain symmetry operations, then so should their material parameters (susceptibility tensors) [44,45].
For example, consider the metasurface in Fig. 3(a), with all possible symmetries: reflection ($\sigma _x$, $\sigma _y$, $\sigma _z$) and rotation ($C_{4,z}$). These symmetries can be used to write invariance conditions on the susceptibility tensors in (8) which eliminate incongruous components. The invariance relations are given in [45] along with an algorithm to easily apply them. Following this algorithm, the hypersusceptiblity matrix reduces to the 9 terms in Fig. 2(c). Furthermore, if the unit cell is deeply subwavelength ($p\ll \lambda$, where $\lambda$ is the wavelength in the background, or the shorter of the two wavelengths in the top or bottom media), then higher-order susceptibilities will be negligible such that the surface can be described using only $\chi _{\text {ee}}^{xx}$, $\chi _{\text {mm}}^{yy}$, and $\chi _{\text {ee}}^{zz}$. Also, if the metasurface is very thin, as in 3(b), then $\chi _{\text {ee}}^{zz}$ may be negligible, such that only $\chi _{\text {ee}}^{xx}$ and $\chi _{\text {mm}}^{yy}$ are necessary.
However, optical meta-atoms are generally large, such that the dipolar model is inappropriate [30]. Then, quadrupolar susceptibilities are necessary, and these provide additional degrees of freedom for specifying wave transformations. To provide even more additional degrees of freedom, spatial symmetries can be broken. For example, consider breaking $\sigma _z$ symmetry, as is the case for the meta-atom in Fig. 3(c). By following the algorithm in [45], one arrives at the matrix with 14 terms in Fig. 2(d). This matrix allows for bianisotropy (e.g. $\chi _\text {em}^{xy}$), and will be used later to demonstrate the utility of the additional degrees of freedom for wave transformations.
4. Synthesis and scattering analysis
Given (4a-b) and (11), it is possible to calculate the fields that will be scattered from a metasurface. In this section, we will consider how plane waves are scattered for a metasurface and how to engineer the susceptibilities to control the angular scattering behaviour.
We will consider TM-polarized plane waves propgagting in the $xz$ plane. With reference Fig. 4, we express the fields as
Now, these fields can be substituted into the GSTCs (4a-b) and the constitutive relations (11). In the case of forward illumination, this provides equations to solve for the two unknowns $S_{11}$ and $S_{21}$, and for backwards illumination one can solve for $S_{22}$ and $S_{21}$. However, the expressions for these S-parameters are very unwieldy, and so we will limit the analysis to some of the terms from Fig. 3. Considering the dipolar susceptibilities $\chi _{\text {ee}}^{xx}$, $\chi _{\text {mm}}^{yy}$, $\chi _{\text {ee}}^{zz}$, then
Meanwhile, for use later, we will also derive expressions for the scattering with $\chi _{\text {em}}^{xy}$, $S_\text {me}^{yzzx}$. We find
Given these expressions, one can solve for the susceptibilities required to control the angular scattering behaviour. For example, to suppress reflection at some angle $k_x^{'}$, one needs to solve $|S_{11}(k_x^{'})|=0$.
Finally, what we have discussed so far only corresponds to the first part of the general metasurface synthesis procedure described in [30,35]. The second part consists in finding the shape of the actual scattering particles, such as those shown in Fig. 3, that would be able to realize the proposed metasurfaces whose scattering parameters are given in (14) and (15). While this work concentrates on the first part of this synthesis procedure, the second part could be achieved by simulating the scattering parameters of the unit cell in Fig. 3 using periodic boundary conditions and for multiple angles of incidence. Then, using in (12), a large system of equations can be formulated that relates these scattering parameters to the metasurface effective hyper-susceptibilities that can then be matched with those of (14) and (15), as detailed in [30,35].
5. Illustration: tuning Brewster’s angle
The Brewster angle is defined as the angle of incidence of a plane wave at a dielectric interface where reflection is eliminated; i.e., there is complete transmission. For ordinary (non-magnetic) materials, it only occurs for TM polarization, and can be understood intuitively from Fig. 5(a). When the angle of incidence is $\theta _\text {i,1}$ and the angle of refraction is $\theta _\text {t,1}$, the wave vectors of the refracted and reflected fields are orthogonal. Consequently, the bulk electric polarization in the substrate is orthogonal to the electric field of the reflected field and it is impossible for the bulk polarization to produce a reflected field. This Brewster angle $\theta _\text {i}=\theta _\text {B}$ occurs at [46]
which corresponds to $k_{x}=k_{\text {B}}=k_1\sin \theta _\text {B}$.Using a metasurface, it is possible to tune $\theta _\text {B}$ [34]. In Fig. 5(b), a metasurface has been added that has a surface polarization which has a non-zero projection onto the reflected electric field at $\theta _\text {i,1}$ and thus the reflection is no longer suppressed. However, now there can be another angle $\theta _\text {i,2}$ where the superposition of the scattered fields from the bulk and the metasurface result in a suppression of the scattered fields, as in Fig. 5(c). By adjusting the metasurface, this angle can be tuned. In fact, we will show that it is possible to have multiple such Brewster angles. There is one caveat: metasurfaces are generally resonant and thus limited in bandwidth unlike the broadband dielectric Brewster effect given by (16).
In this section, we will illustrate the use of the additional susceptibility components from Fig. 2(d) to achieve this generalized Brewster effect.
5.1 Generalized Brewster effect
Consider the very simple case of a Huygen’s metasurface with $\chi _{\text {ee}}^{xx}$ and $\chi _{\text {mm}}^{yy}$. Using these two terms, it is possible to achieve a single wave transformation [23], which we would desire to be the suppression of reflection at a given angle of incidence. This corresponds to impedance matching the two media at a given angle. We will ensure that the metasurface is lossless, which will ensure that all power is transmitted. Setting $|S_{11}|=0$ in (14) and solving for $\chi _{\text {ee}}^{xx}$, we find
Figure 6(a) shows $\Im \{\chi _{\text {ee}}^{xx}\}$ plotted as a function of the angle of incidence ($k_x/k_0$) on the $x$-axis and $\chi _{\text {mm}}^{yy}$ on the $y$-axis, for a particular case where a plane wave is incident from air ($\epsilon _1=1$) onto a substrate ($\epsilon _2=2$). Consider in particular the black contours along which $\Im \{\chi _{\text {ee}}^{xx}\}=0$. Choosing a point along these contours corresponds to a lossless and gainless metasurface. Next, Fig. 6(b) shows the same contours superimposed on a plot of $\Re \{\chi _{\text {ee}}^{xx}\}$. We see that the contours cover all incident angles ($-k_0<k_x<k_0$). Thus, one can choose any angle of incidence and the necessary susceptibilities to achieve a Brewster effect at the given angle. For example, to achieve $k_\text {B}=0.6k_0$, $\chi _{\text {ee}}^{xx}={4.44}\times 10^{-4}{m}$ and $\chi _{\text {mm}}^{yy}={2.28}\times 10^{-4}{m}$. The corresponding reflected and transmitted power is plotted in Fig. 6(c), corroborating a Brewster angle at $k_\text {B}=0.6k_0$. Note that for the transmitted power, an angle-dependent factor is used in $(\cos \theta _2/\cos \theta _1)|S_{21}|^2$ to project the Poynting vector to $\mathbf {\hat {z}}$ [35]. To practically realize such a metasurface, one could use the cell in Fig. 3(b).
Now, we will consider other susceptibility terms to demonstrate how the additional degrees of freedom provide more control over the Brewster effect. Motivated by the scattering caused by $\chi _{\text {ee}}^{zz}$, which is proportional to $\sin ^2(\theta _\text {B})\cdot \chi _{\text {ee}}^{zz}$ (unlike $\cos ^2(\theta _\text {B})\cdot \chi _{\text {ee}}^{xx}$ and $1\cdot \chi _{\text {mm}}^{yy}$), which can be deduced from (14), let us consider the combination of $\chi _{\text {ee}}^{zz}$ and $\chi _{\text {ee}}^{xx}$. This could be achieved using a meta-atom like that in Fig. 3(a) although $\chi _{\text {mm}}^{yy}$ may in general be present as well but it will typically have a Lorentzian wavelength dependence such that the metasurface can be designed to operate at a frequency where it is negligible [35].
In this case, setting $|S_{11}|=0$ in (14) and solving for $\chi _{\text {ee}}^{zz}$, we find
Finally, we consider the use of quadrupolar susceptibilities. Using the meta-atom of Fig. 3(c), many terms are possible. To demonstrate the versatility of these terms, we will apply two in particular: $S_\text {me}^{yzzx}$ and $\chi _{\text {em}}^{xy}$. Note that we assume all other terms but these two are negligible and we leave the design of such a metasurface, which is not a trivial task, as future work. This time, setting $|S_{11}|=0$ in (15) and solving for $\chi _{\text {em}}^{xy}$, one finds
5.2 Engineered angular reflection (“anti-Brewster”)
To further demonstrate the capabilities of the proposed modeling approach for controlling the angular scattering response of a multipolar metasurface, we shall now consider the case of engineered angular reflection for which the transmittance goes to zero.
In addition to suppressing reflection at a particular angle to control the Brewster angle, it is possible to suppress transmission to create what we will call an “anti-Brewster” angle. We will consider the same sets of susceptibilities as in Section 5. Starting with $\chi _{\text {ee}}^{xx}$ and $\chi _{\text {mm}}^{yy}$ in (15), setting $|S_{21}|=0$, and solving for the susceptibilities,
which has no dependence on the angle of incidence ($k_x$, $k_{z,1}$, or $k_{z,2}$). Thus, if (20) is satisfied, the metasurface will behave as a mirror with complete reflection, rather than the desired refection at a particular angle of incidence.Thus, we again consider $\chi _{\text {ee}}^{zz}$, due to its angular behavior, along with $\chi _{\text {ee}}^{xx}$. Then, the condition for complete reflection is
which has a dependence on $k_x$. Designing for $k_x=0.6k_0$, Fig. 8(a) shows the reflected and transmitted powers, verifying the “anti-Brewster” behavior.Finally, we consider quadrupolar susceptibilities. With $S_\text {me}^{yzzx}$ and $\chi _{\text {em}}^{xy}$, there are two solutions for suppressed transmission:
Overall, we see that by adding more susceptibility terms – and terms relating to quadrupoles and spatial disperion in particular – it is possible to have increasing control over the angular scattering response. While we have highlighted a few of the possible terms in the general hypersusceptibity matrix (8), other susceptibilities could be considered for even more intricate control, such as more Brewster or “anti-Brewster” angles.
6. Conclusion
In summary, we have derived GSTCs which include spatial dispersion and are valid for metasurfaces in non-homogeneous environments, such as for practical metasurfaces fabricated on a substrate. We have shown how the susceptiblity tensor properties (symmetries, reciprocity, tracelessness) and spatial symmetries of the metasurface can be used to simplify the susceptibility tensors. Furthermore, we demonstrated how the new hyper-susceptibility terms can be used to produce multiple Brewster and “anti-Brewster” angles. For example, with tuning of $\chi _{\text {em}}^{xy}$ and $S_\text {me}^{yzzx}$ it is possible to achieve 3 Brewster angles and 2 “anti-Brewster” angles. We expect this work to provide a fundamental advance for Fourier-domain signal processing, where tuning of the angular response is paramount.
Funding
Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung (PZ00P2_193221).
Disclosures
The authors declare no conflicts of interest.
Data availability
Data underlying the results presented in this paper are not publicly available at this time but may be obtained from the authors upon reasonable request.
Supplemental document
See Supplement 1 for supporting content.
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