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Ultrafast photo-induced melting of the trimer superstructure in TaTe2

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Abstract

We report the first ultrafast study of TaTe2, utilizing MeV-scale ultrafast electron diffraction to reveal rapid photo-induced melting of its low-temperature trimer superstructure. Density-functional calculations indicate intra-trimer charge transfer as a trigger of this transformation.

© 2021 The Author(s)

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