Abstract

We have developed a nonperturbative analytical approach to the problem of the interaction of high-power chirped ultrashort pulses with molecular systems. We have considered a molecule with two electronic states in a solvent interacting with a strong chirped pulse, whose field amplitude can be represented in the form: $E\left(t\right)=ℰ\left(t\right)\exp \left(i\phi \left(t\right)\right)$, where $ℰ\left(t\right)$ and φ(t) are real functions of time. We consider the case when the electron-vibrational interaction can be described as a Gaussian-Markovian process.

© 1998 IEEE