Stochastic Dynamics of a Single Laser-Driven Molecule with Double Well Potentials in Ground and Excited Electronic States

S. Ya. Kilin; A. P. Nizovtsev; T. M. Maevskaya; V. N. Shatokhin; P. R. Berman; J. Wrachtrup; L. Fleury; C. von Borczyskowski

European Quantum Electronics Conference
Technical Digest Series (Optica Publishing Group, 1998),
paper QThK1

Stochastic Dynamics of a Single Laser-Driven Molecule with Double Well Potentials in Ground and Excited Electronic States

S. Ya. Kilin, A. P. Nizovtsev, T. M. Maevskaya, V. N. Shatokhin, P. R. Berman, J. Wrachtrup, L. Fleury, and C. von Borczyskowski

European Quantum Electronics Conference 1998

Glasgow, Scotland United Kingdom
14–18 September 1998
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Lasers in Chemistry: Solids and Gases (QThK)

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S. Y. Kilin, A. P. Nizovtsev, T. M. Maevskaya, V. N. Shatokhin, P. R. Berman, J. Wrachtrup, L. Fleury, and C. von Borczyskowski, "Stochastic Dynamics of a Single Laser-Driven Molecule with Double Well Potentials in Ground and Excited Electronic States," in European Quantum Electronics Conference, Technical Digest Series (Optica Publishing Group, 1998), paper QThK1.

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Abstract

We have studied stochastic jumps in a laser-excited fluorescence emitted by a single molecule having double well potentials (DWP) in ground and excited electronic states. This molecule model is rather general and applicable to a variety of condensed-matter, chemical and biological systems, probed by fluorescence excitation. The specific examples considered are (i) a single guest chromophore molecule strongly coupled to a nearby single asymmetric structural two-level system (TLS) in embedding amorphous host matrix and (ii) a single point defect in crystalline solids whose DWP’s are due to existence of two possible configurations of a defect.

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