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Separating the direct and cascaded contributions to two-dimensional Raman signals using phase-sensitive detection

O. Golonzka, N. Demirdttven, and A. Tokmakoff

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Abstract

We demonstrate a method of phase-sensitive detection for separating the direct and the cascaded contributions to fifth-order 2-D Raman spectroscopy. The phase of an intrinsic local oscillator is cycled to distinguish the two components that are radiated in quadrature to each other.

© 2000 Optical Society of America

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