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Ultrafast Vibrational Relaxation of Excited Free OD at the Air/Water Interface Revealed by Femtosecond Time-Resolved HD-VSFG spectroscopy

Mohammed Ahmed, Satoshi Nihonyanagi, and Tahei Tahara

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Abstract

Femtosecond time-resolved HD-VSFG spectroscopy reveals ultrafast vibrational dynamics of free OD at the air/water interface. The absence of isotope dilution effect on the vibrational lifetime suggests that the excited free OD relaxes predominantly through the reorientation mechanism.

© 2022 The Author(s)

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